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Dry-Scrubbing of Acid Gases in Recirculating Cyclones

dc.contributor.authorChibante, Vaniapor
dc.contributor.authorFonseca, Ana
dc.contributor.authorSalcedo, Romualdo
dc.date.accessioned2007-10-02T08:26:42Zpor
dc.date.accessioned2011-10-06T14:40:38Z
dc.date.available2007-10-02T08:26:42Zpor
dc.date.available2011-10-06T14:40:38Z
dc.date.issued2007por
dc.description.abstractThis paper describes a laboratory-scale study on the use of recirculating cyclones as reaction chambers for dry scrubbing of gaseous HCl with solid slaked lime particles. This gas cleaning system combines a numerically optimized reverse flow gas cyclone (RS_VHE geometry) with a straight-through cyclone concentrator, which simultaneously increases the capture of the solid particles and promotes their partial recirculation. A laboratory-scale study was undertaken to test this technology and to compare its performance to a modified Stairmand HE reverse flow cyclone without recirculation. The experimental conditions were: reaction temperature ≈326K, gas flow rate ≈2.9x10-4Nm3.s-1 and relative humidity of the gas ≈8.5%. The experimental variables tested were the solids load (1.0-9.2 x10-7kg.s-1) and HCl concentration (0.4-2.8 x10-2mol.m-3) in the inlet gas. The experimentally obtained particulate removal efficiencies with the recirculating cyclones (≈98%) were higher than those obtained with the Stairmand HE cyclone (≈93%), with the additional advantage of having significantly lower pressure drop. As for the acid removal efficiencies (≈10 to 96%), no significant differences were found between the two systems tested under the same experimental conditions. The possibility of using optimized recirculating cyclones for gas cleaning in a dry scrubbing process is very promising, since this is a low cost technology, highly efficient both for the removal of acid gases and for the capture of solid particles, which has the advantage of not requiring a post-reaction de-duster.por
dc.description.sponsorshipThe authors acknowledge the financial support from the Portuguese Foundation for Science and Technology (FCT) through the contract POCTI/EQU/37992/2001/FEDER and the scholarship BD 8191/2002por
dc.identifier.citationJournal Hazardous Materials. 144 (2007), pp. 682-686.por
dc.identifier.urihttp://hdl.handle.net/10284/294por
dc.language.isoengpor
dc.publisherElsevierpor
dc.relation.ispartofseriesJournal Hazardous Materialspor
dc.relation.ispartofseries144por
dc.subjectRecirculating cyclonespor
dc.subjectGas Cleaningpor
dc.subjectDry-scrubbingpor
dc.subjectHClpor
dc.subjectSlaked limepor
dc.subjectCyclone reactorpor
dc.titleDry-Scrubbing of Acid Gases in Recirculating Cyclonespor
dc.typejournal article
dspace.entity.typePublication
person.familyNameFonseca
person.familyNameSalcedo
person.givenNameAna
person.givenNameRomualdo
person.identifier.ciencia-idF61F-23C0-BBF5
person.identifier.ciencia-idC816-985C-014C
person.identifier.orcid0000-0002-3207-4819
person.identifier.orcid0000-0003-3546-7404
person.identifier.ridG-5355-2013
person.identifier.scopus-author-id7101964374
person.identifier.scopus-author-id7007047524
rcaap.rightsopenAccesspor
rcaap.typearticlepor
relation.isAuthorOfPublication1f238a52-936a-454d-8146-9418c538eea0
relation.isAuthorOfPublicationf77be778-2721-424a-a6e4-f7842d3f164d
relation.isAuthorOfPublication.latestForDiscovery1f238a52-936a-454d-8146-9418c538eea0

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